No. mergerfs is not intended as a form of RAID1. It would overly complicate the design (you'd need logic on how many files to write among other information) and is dangerous given the difficulty in managing error conditions.
Such behavior is better handled with an out of band script. I've considered putting one together but haven't gotten around to it.
If you only have two drives you could easily use rsync to dup between the drives.
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